In 2001, Gotye started recording his initial tracks using samples. He made about 50 copies of his first collection and sent the CDs out to almost every radio station. Feedback was mainly positive with youth orientated radio station Triple J taking notice and giving him confidence to continue with his sample-based recordings.
Gotye met singer Kris Schroeder at a party and the duo started performing under the name The Basics. The two became regulars on the live music scene and went on to release four studio albums between 2004 and 2010.
Gotye was eventually offered a deal by the label Creative Vibes which released an album featuring a collection of songs from his earlier releases. This album was titled ‘Boardface’ (2003).
In the ensuing years, he continued performing with The Basics and also recorded his own songs. He moved numerous times, each time relocating his home recording studio to a new place with new acoustic qualities.
Gotye came up with his second album ‘Like Drawing Blood’ (2006) which commenced his professional relationship with manager Danny Rogers. In 2006, the album was voted the No. 1 album in a listener poll and also earned a J Award nomination. Two singles from the album, "Hearts a Mess" and "Learnalilgivinanlovin," were ranked #8 and #94 respectively in Triple J's Hottest 100 list of 2006.
In the year 2007, Gotye won the ARIA Music Award for best male artist. The following year, his album ‘Like Drawing Blood’ was named iTunes album of the year in UK.
His first European success came in the year 2008 when the singles "Hearts a Mess" and “Learnalilgivinanlovin" charted in Belgium. Soon, ‘Like Drawing Blood’ regained its position in the ARIA charts, peaking at # 13.
In 2010, the Australian artiste released a new track titled "Eyes Wide Open" online. The single garnered positive reviews and peaked at #25 on the Triple J Hottest 100 that year.
Gotye released his album ‘Making Mirrors’ in Australia on August 19, 2011. The album peaked at #1 on the ARIA albums chart within the week of release, making him the first Australian to concurrently hold the No. 1 album and single since Silverchair in 2007.
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’Making Mirrors’ later became a success worldwide, peaking at #1 in numerous countries and gaining a spot in the top 10 in several others. The album earned gold status in USA, Germany, New Zealand, UK, Canada, Ireland and the Netherlands, and platinum in Poland, France and Belgium, and 3x platinum in Australia.
On 18 October 2011, Gotye came up a video clip for the track "Don't Worry, We'll Be Watching You" on Vimeo and YouTube.
In 2012, he made his American television debut when he appeared on ‘Jimmy Kimmel Live!’ and performed some of his hit songs. In February 2012, he released the music video of "Easy Way Out" online. In August, he commenced his world tour, starting from Korea and covering Japan, Europe North America and finishing in Australia.
In early 2013, Gotye collaborated with illuminart to launch ‘Fractured Heart,’ a sound and light sculpture at National Film and Sound Archive headquarters in Canberra, Australia.
In 2014, he launched the independent record label Spirit Level with Tim Shiel. Gotye also remained active as a singer and drummer of The Basics, releasing ‘The Lucky Country’ and ‘The Age of Entitlement.’
He was a featured vocalist on the English musician Bibio's single "The Way You Talk" on his 2016 album ‘A Mineral Love.’
Gotye became friends with Jean-Jacques Perrey in the mid-2010s and worked with him to preserve his recorded legacy. Gotye, along with five other members, then formed the Ondioline Orchestra in New York. They made their debut on 22 November 2016, performing two shows in tribute to Jean-Jacques Perrey at the National Sawdust in Brooklyn.
In May 2017, Gotye launched a new record label called Forgotten Futures. A year later, his Ondioline Orchestra paid a tribute to Perrey at the Roulette's Mixology Festival 2018.